People
Visiting Research Professors & Research Fellow
Makars Šiškins
Title
Visiting Research Fellow
Degree
PhD
Research Interests
Graphene, 2D materials, nanomechanics, magnetism, high-temperature electronics
Biography
Lecturer in Experimental Physics – School of Physics and Astronomy, University of Southampton
Selected Publications
- I. E. Rosłoń, R. J. Dolleman, H. Licona, M. Lee, M. Šiškins, H. Lebius, L. Madauß, M. Schleberger, F. Alijani, H. S. J. van der Zant, and P. G. Steeneken. High-frequency gas effusion through nanopores in suspended graphene. Nature Communications, 11 (6025), 1, 2020, DOI: 10.1038/s41467-020-19893-5
- Makars Šiškins, Martin Lee, Samuel Mañas-Valero, Eugenio Coronado, Yaroslav M. Blanter, Herre S. J. van der Zant, and Peter G. Steeneken. Magnetic and electronic phase transitions probed by nanomechanical resonators. Nature Communications, 11 (2698), 1, 2020 DOI: 10.1038/s41467-020-16430-2
- Makars Šiškins, Martin Lee, Farbod Alijani, Mark R. van Blankenstein, Dejan Davidovikj, Herre S. J. van der Zant, and Peter G. Steeneken. Highly Anisotropic Mechanical and Optical Properties of 2D Layered As2S3 Membranes. ACS Nano, 13 (9), 10845–10851, 2019, DOI: 10.1021/acsnano.9b06161
I-FIM Publications:
2025 |
Fullerton, John; Li, Yue; Solanki, Harshvardhan; Grebenchuk, Sergey; Grzeszczyk, Magdalena; Chen, Zhaolong; Siskins, Makars; Novoselov, Kostya S; Koperski, Maciej; Santos, Elton J G; Phatak, Charudatta Observation of Topological Chirality Switching Induced Freezing of a Skyrmion Crystal ADVANCED MATERIALS, 2025, DOI: 10.1002/adma.202513067. @article{WOS:001601237600001, title = {Observation of Topological Chirality Switching Induced Freezing of a Skyrmion Crystal}, author = {John Fullerton and Yue Li and Harshvardhan Solanki and Sergey Grebenchuk and Magdalena Grzeszczyk and Zhaolong Chen and Makars Siskins and Kostya S Novoselov and Maciej Koperski and Elton J G Santos and Charudatta Phatak}, doi = {10.1002/adma.202513067}, times_cited = {0}, issn = {0935-9648}, year = {2025}, date = {2025-10-01}, journal = {ADVANCED MATERIALS}, publisher = {WILEY-V C H VERLAG GMBH}, address = {POSTFACH 101161, 69451 WEINHEIM, GERMANY}, abstract = {Magnetic skyrmions are topologically protected quasi-particles with a well-defined chirality. Control over their chirality is proposed as an additional feature for encoding data bits or as qubits in quantum computing due to their high efficiency and stability against achiral magnetic textures. Here it is shown that an in-plane magnetic field can be utilized to reshape the energy barriers between different skyrmionic bubbles (e.g., Bloch type, type-II) enabling spontaneous chirality fluctuations with a frequency that increases with the strength of the in-plane field. The insulating van der Waals ferromagnet CrBr3 is used as an archetypal system for low damping, reduced energy dissipation and a high number of magnetic phases to capture the chirality dynamics in real time through cryo-Lorentz transmission electron microscopy. It is observed that the interplay between the intrinsic Dzyaloshinskii-Moriya interaction and out-of-plane field biased the chirality dynamics, favoring one handedness over the other. A remarkable consequence of the spontaneous chirality switching mechanism is that it induces a freezing (or crystallization) process in the skyrmion lattice. As the bubbles fluctuate between Bloch and type-II they elongate and shrink parallel to the in-plane field. Subsequently, the overall lattice crystallizes along the in-plane field direction, inducing a phase transition from a disordered liquid state to a hexatic phase where skyrmions are highly ordered resembling that of a solid. The results indicate chirality as an active element in the creation of topologically protected skyrmion crystals unveiling pathways toward chiral spintronic device platforms with tunable embedded configuration.}, keywords = {}, pubstate = {published}, tppubtype = {article} } Magnetic skyrmions are topologically protected quasi-particles with a well-defined chirality. Control over their chirality is proposed as an additional feature for encoding data bits or as qubits in quantum computing due to their high efficiency and stability against achiral magnetic textures. Here it is shown that an in-plane magnetic field can be utilized to reshape the energy barriers between different skyrmionic bubbles (e.g., Bloch type, type-II) enabling spontaneous chirality fluctuations with a frequency that increases with the strength of the in-plane field. The insulating van der Waals ferromagnet CrBr3 is used as an archetypal system for low damping, reduced energy dissipation and a high number of magnetic phases to capture the chirality dynamics in real time through cryo-Lorentz transmission electron microscopy. It is observed that the interplay between the intrinsic Dzyaloshinskii-Moriya interaction and out-of-plane field biased the chirality dynamics, favoring one handedness over the other. A remarkable consequence of the spontaneous chirality switching mechanism is that it induces a freezing (or crystallization) process in the skyrmion lattice. As the bubbles fluctuate between Bloch and type-II they elongate and shrink parallel to the in-plane field. Subsequently, the overall lattice crystallizes along the in-plane field direction, inducing a phase transition from a disordered liquid state to a hexatic phase where skyrmions are highly ordered resembling that of a solid. The results indicate chirality as an active element in the creation of topologically protected skyrmion crystals unveiling pathways toward chiral spintronic device platforms with tunable embedded configuration.
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Grebenchuk, Sergey Y; Grzeszczyk, Magdalena; Chen, Zhaolong; Siskins, Makars; Borisov, Vladislav; Pereiro, Manuel; Katsnelson, Mikhail I; Eriksson, Olle; Novoselov, Kostya S; Koperski, Maciej Correlations in Magnetic Sub-Domains as an Unconventional Phase Diagram for van der Waals Ferromagnets ADVANCED SCIENCE, 12 (26), 2025, DOI: 10.1002/advs.202500562. @article{WOS:001464532700001, title = {Correlations in Magnetic Sub-Domains as an Unconventional Phase Diagram for van der Waals Ferromagnets}, author = {Sergey Y Grebenchuk and Magdalena Grzeszczyk and Zhaolong Chen and Makars Siskins and Vladislav Borisov and Manuel Pereiro and Mikhail I Katsnelson and Olle Eriksson and Kostya S Novoselov and Maciej Koperski}, doi = {10.1002/advs.202500562}, times_cited = {2}, year = {2025}, date = {2025-07-01}, journal = {ADVANCED SCIENCE}, volume = {12}, number = {26}, publisher = {WILEY}, address = {111 RIVER ST, HOBOKEN 07030-5774, NJ USA}, abstract = {Traditional magnetic phase diagram represents a transition between the ferromagnetic and paramagnetic states of a material under the influence of varied temperature, magnetic field, and pressure. So far, the ferromagnetic phase has been considered predominantly as a single type of magnetization texture extending macroscopically in the bulk of a crystal, existing as a ground state determined by the interactions between localized magnetic moments arranged in a lattice. Here, it is demonstrated that an unconventional magnetic order composed of vertically correlated planar magnetic sub-domains occurs intrinsically in mechanically exfoliated layers of van der Waals ferromagnet CrBr3. Based on the visualization of the magnetic textures through magnetic force microscopy in conjunction with the ab initio calculations of the crystal structure in the magnetic phase and micromagnetic simulations, the origin of the magnetic sub-domains is attributed to stacking faults isolating a van der Waals ferromagnetic well from the bulk film due to modifications in the interlayer exchange coupling. This enables to create a phase diagram describing the magnetic states unique to van der Waals ferromagnets in terms of the degree of correlation between the magnetic sub-domains, dependent on the exchange coupling constants and tuneable by magnetic field and temperature.}, keywords = {}, pubstate = {published}, tppubtype = {article} } Traditional magnetic phase diagram represents a transition between the ferromagnetic and paramagnetic states of a material under the influence of varied temperature, magnetic field, and pressure. So far, the ferromagnetic phase has been considered predominantly as a single type of magnetization texture extending macroscopically in the bulk of a crystal, existing as a ground state determined by the interactions between localized magnetic moments arranged in a lattice. Here, it is demonstrated that an unconventional magnetic order composed of vertically correlated planar magnetic sub-domains occurs intrinsically in mechanically exfoliated layers of van der Waals ferromagnet CrBr3. Based on the visualization of the magnetic textures through magnetic force microscopy in conjunction with the ab initio calculations of the crystal structure in the magnetic phase and micromagnetic simulations, the origin of the magnetic sub-domains is attributed to stacking faults isolating a van der Waals ferromagnetic well from the bulk film due to modifications in the interlayer exchange coupling. This enables to create a phase diagram describing the magnetic states unique to van der Waals ferromagnets in terms of the degree of correlation between the magnetic sub-domains, dependent on the exchange coupling constants and tuneable by magnetic field and temperature.
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Bermejillo-Seco, Alvaro; Zhang, Xiang; Houmes, Maurits J A; Siskins, Makars; van der Zant, Herre S J; Steeneken, Peter G; Blanter, Yaroslav M Thermoelastic damping across the phase transition in van der Waals magnets PHYSICAL REVIEW B, 111 (24), 2025, DOI: 10.1103/PhysRevB.111.245409. @article{WOS:001511202800006, title = {Thermoelastic damping across the phase transition in van der Waals magnets}, author = {Alvaro Bermejillo-Seco and Xiang Zhang and Maurits J A Houmes and Makars Siskins and Herre S J van der Zant and Peter G Steeneken and Yaroslav M Blanter}, doi = {10.1103/PhysRevB.111.245409}, times_cited = {1}, issn = {2469-9950}, year = {2025}, date = {2025-06-01}, journal = {PHYSICAL REVIEW B}, volume = {111}, number = {24}, publisher = {AMER PHYSICAL SOC}, address = {ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA}, abstract = {A quantitative understanding of the microscopic mechanisms responsible for damping in van der Waals nanomechanical resonators remains elusive. In this work, we investigate van der Waals magnets, where the thermal expansion coefficient exhibits an anomaly at the magnetic phase transition due to magnetoelastic coupling. Thermal expansion mediates the coupling between mechanical strain and heat flow and determines the strength of thermoelastic damping (TED). Consequently, variations in the thermal expansion coefficient are reflected directly in TED, motivating our focus on this mechanism. We extend existing TED models to incorporate anisotropic thermal conduction, a critical property of van der Waals materials. By combining the thermodynamic properties of the resonator material with the anisotropic TED model, we examine dissipation as a function of temperature. Our findings reveal a pronounced impact of the phase transition on dissipation, along with transitions between distinct dissipation regimes controlled by geometry and the relative contributions of in-plane and out-of-plane thermal conductivity. These regimes are characterized by the resonant interplay between strain and in-plane or through-plane heat propagation. To validate our theory, we compare it to experimental data of the temperature-dependent mechanical resonances of FePS3 resonators.}, keywords = {}, pubstate = {published}, tppubtype = {article} } A quantitative understanding of the microscopic mechanisms responsible for damping in van der Waals nanomechanical resonators remains elusive. In this work, we investigate van der Waals magnets, where the thermal expansion coefficient exhibits an anomaly at the magnetic phase transition due to magnetoelastic coupling. Thermal expansion mediates the coupling between mechanical strain and heat flow and determines the strength of thermoelastic damping (TED). Consequently, variations in the thermal expansion coefficient are reflected directly in TED, motivating our focus on this mechanism. We extend existing TED models to incorporate anisotropic thermal conduction, a critical property of van der Waals materials. By combining the thermodynamic properties of the resonator material with the anisotropic TED model, we examine dissipation as a function of temperature. Our findings reveal a pronounced impact of the phase transition on dissipation, along with transitions between distinct dissipation regimes controlled by geometry and the relative contributions of in-plane and out-of-plane thermal conductivity. These regimes are characterized by the resonant interplay between strain and in-plane or through-plane heat propagation. To validate our theory, we compare it to experimental data of the temperature-dependent mechanical resonances of FePS3 resonators.
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Siskins, Makars; Keskekler, Ata; Houmes, Maurits J A; Manas-Valero, Samuel; Koperski, Maciej; Coronado, Eugenio; Blanter, Yaroslav M; van der Zant, Herre S J; Steeneken, Peter G; Alijani, Farbod Nonlinear dynamics and magneto-elasticity of nanodrums near the phase transition NATURE COMMUNICATIONS, 16 (1), 2025, DOI: 10.1038/s41467-025-57317-4. @article{WOS:001443899000027, title = {Nonlinear dynamics and magneto-elasticity of nanodrums near the phase transition}, author = {Makars Siskins and Ata Keskekler and Maurits J A Houmes and Samuel Manas-Valero and Maciej Koperski and Eugenio Coronado and Yaroslav M Blanter and Herre S J van der Zant and Peter G Steeneken and Farbod Alijani}, doi = {10.1038/s41467-025-57317-4}, times_cited = {4}, year = {2025}, date = {2025-03-01}, journal = {NATURE COMMUNICATIONS}, volume = {16}, number = {1}, publisher = {NATURE PORTFOLIO}, address = {HEIDELBERGER PLATZ 3, BERLIN, 14197, GERMANY}, abstract = {Nanomechanical resonances of two-dimensional (2D) materials are sensitive probes for condensedmatter physics, offering new insights into magnetic and electronic phase transitions. Despite extensive research, the influence of the spin dynamics near a phase transition on the nonlinear dynamics of 2D membranes has remained largely unexplored. Here, we investigate nonlinear magneto-mechanical coupling to antiferromagnetic order in suspended FePS3-based heterostructure membranes. By monitoring the motion of these membranes as a function of temperature, we observe characteristic features in both nonlinear stiffness and damping close to the N & eacute;el temperature TN. We account for these experimental observations with an analytical magnetostriction model in which these nonlinearities emerge from a coupling between mechanical and magnetic oscillations, demonstrating that magneto-elasticity can lead to nonlinear damping. Our findings thus provide insights into the thermodynamics and magneto-mechanical energy dissipation mechanisms in nanomechanical resonators due to the material's phase change and magnetic order relaxation.}, keywords = {}, pubstate = {published}, tppubtype = {article} } Nanomechanical resonances of two-dimensional (2D) materials are sensitive probes for condensedmatter physics, offering new insights into magnetic and electronic phase transitions. Despite extensive research, the influence of the spin dynamics near a phase transition on the nonlinear dynamics of 2D membranes has remained largely unexplored. Here, we investigate nonlinear magneto-mechanical coupling to antiferromagnetic order in suspended FePS3-based heterostructure membranes. By monitoring the motion of these membranes as a function of temperature, we observe characteristic features in both nonlinear stiffness and damping close to the N & eacute;el temperature TN. We account for these experimental observations with an analytical magnetostriction model in which these nonlinearities emerge from a coupling between mechanical and magnetic oscillations, demonstrating that magneto-elasticity can lead to nonlinear damping. Our findings thus provide insights into the thermodynamics and magneto-mechanical energy dissipation mechanisms in nanomechanical resonators due to the material's phase change and magnetic order relaxation.
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2024 |
Grebenchuk, Sergey; Mckeever, Conor; Grzeszczyk, Magdalena; Chen, Zhaolong; Siskins, Makars; McCray, Arthur R C; Li, Yue; Petford-Long, Amanda K; Phatak, Charudatta M; Ruihuan, Duan; Zheng, Liu; Novoselov, Kostya S; Santos, Elton J G; Koperski, Maciej Topological Spin Textures in an Insulating van der Waals Ferromagnet 24 ADVANCED MATERIALS, 36 (24), 2024, DOI: 10.1002/adma.202311949. @article{WOS:001177264100001, title = {Topological Spin Textures in an Insulating van der Waals Ferromagnet}, author = {Sergey Grebenchuk and Conor Mckeever and Magdalena Grzeszczyk and Zhaolong Chen and Makars Siskins and Arthur R C McCray and Yue Li and Amanda K Petford-Long and Charudatta M Phatak and Duan Ruihuan and Liu Zheng and Kostya S Novoselov and Elton J G Santos and Maciej Koperski}, doi = {10.1002/adma.202311949}, times_cited = {24}, issn = {0935-9648}, year = {2024}, date = {2024-06-01}, journal = {ADVANCED MATERIALS}, volume = {36}, number = {24}, publisher = {WILEY-V C H VERLAG GMBH}, address = {POSTFACH 101161, 69451 WEINHEIM, GERMANY}, abstract = {Generation and control of topological spin textures constitutes one of the most exciting challenges of modern spintronics given their potential applications in information storage technologies. Of particular interest are magnetic insulators, which due to low damping, absence of Joule heating and reduced dissipation can provide energy-efficient spin-textures platform. Here, it is demonstrated that the interplay between sample thickness, external magnetic fields, and optical excitations can generate a prolific paramount of spin textures, and their coexistence in insulating CrBr3 van der Waals (vdW) ferromagnets. Using high-resolution magnetic force microscopy and large-scale micromagnetic simulation methods, the existence of a large region in T-B phase diagram is demonstrated where different stripe domains, skyrmion crystals, and magnetic domains exist and can be intrinsically selected or transformed to each-other via a phase-switch mechanism. Lorentz transmission electron microscopy unveils the mixed chirality of the magnetic textures that are of Bloch-type at given conditions but can be further manipulated into Neel-type or hybrid-type via thickness-engineering. The topological phase transformation between the different magnetic objects can be further inspected by standard photoluminescence optical probes resolved by circular polarization indicative of an existence of exciton-skyrmion coupling mechanism. The findings identify vdW magnetic insulators as a promising framework of materials for the manipulation and generation of highly ordered skyrmion lattices relevant for device integration at the atomic level. The formation of a skyrmion lattice in van der Waals ferromagnet CrBr3 opens pathways for exploration of topological spin textures in 2D insulating crystals. These skyrmions manifest in unusual crystalline environment characterized by centrosymmetric crystal structure and are stabilized through dipolar rather than Dzyaloshinskii-Moriya interactions. The construction of B-T phase diagram enables versatile phase-switching mechanisms for controlling magnetization textures. image}, keywords = {}, pubstate = {published}, tppubtype = {article} } Generation and control of topological spin textures constitutes one of the most exciting challenges of modern spintronics given their potential applications in information storage technologies. Of particular interest are magnetic insulators, which due to low damping, absence of Joule heating and reduced dissipation can provide energy-efficient spin-textures platform. Here, it is demonstrated that the interplay between sample thickness, external magnetic fields, and optical excitations can generate a prolific paramount of spin textures, and their coexistence in insulating CrBr3 van der Waals (vdW) ferromagnets. Using high-resolution magnetic force microscopy and large-scale micromagnetic simulation methods, the existence of a large region in T-B phase diagram is demonstrated where different stripe domains, skyrmion crystals, and magnetic domains exist and can be intrinsically selected or transformed to each-other via a phase-switch mechanism. Lorentz transmission electron microscopy unveils the mixed chirality of the magnetic textures that are of Bloch-type at given conditions but can be further manipulated into Neel-type or hybrid-type via thickness-engineering. The topological phase transformation between the different magnetic objects can be further inspected by standard photoluminescence optical probes resolved by circular polarization indicative of an existence of exciton-skyrmion coupling mechanism. The findings identify vdW magnetic insulators as a promising framework of materials for the manipulation and generation of highly ordered skyrmion lattices relevant for device integration at the atomic level. The formation of a skyrmion lattice in van der Waals ferromagnet CrBr3 opens pathways for exploration of topological spin textures in 2D insulating crystals. These skyrmions manifest in unusual crystalline environment characterized by centrosymmetric crystal structure and are stabilized through dipolar rather than Dzyaloshinskii-Moriya interactions. The construction of B-T phase diagram enables versatile phase-switching mechanisms for controlling magnetization textures. image
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